Charge ordering, ferroelectric, and magnetic domains in LuFe2O4 observed by scanning probe microscopy

I. K. Yang, Jeehoon Kim, S. H. Lee, Sang-Wook Cheong, Y. H. Jeong

Research output: Contribution to journalArticle

10 Citations (Scopus)

Abstract

LuFe2O4 is a multiferroic system which exhibits charge order, ferroelectricity, and ferrimagnetism simultaneously below ∼230 K. The ferroelectric/charge order domains of LuFe2O4 are imaged with both piezoresponse force microscopy (PFM) and electrostatic force microscopy (EFM), while the magnetic domains are characterized by magnetic force microscopy (MFM). Comparison of PFM and EFM results suggests that the proposed ferroelectricity in LuFe2O4 is not of usual displacive type but of electronic origin. Simultaneous characterization of ferroelectric/charge order and magnetic domains by EFM and MFM, respectively, on the same surface of LuFe2O4 reveals that both domains have irregular patterns of similar shape, but the length scales are quite different. The domain size is approximately 100 nm for the ferroelectric domains, while the magnetic domain size is much larger and gets as large as 1 μm. We also demonstrate that the origin of the formation of irregular domains in LuFe2O4 is not extrinsic but intrinsic.

Original languageEnglish (US)
Article number152902
JournalApplied Physics Letters
Volume106
Issue number15
DOIs
StatePublished - Apr 13 2015

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magnetic domains
microscopy
scanning
probes
magnetic force microscopy
ferroelectricity
electrostatics
ferrimagnetism
electronics

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy (miscellaneous)

Cite this

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abstract = "LuFe2O4 is a multiferroic system which exhibits charge order, ferroelectricity, and ferrimagnetism simultaneously below ∼230 K. The ferroelectric/charge order domains of LuFe2O4 are imaged with both piezoresponse force microscopy (PFM) and electrostatic force microscopy (EFM), while the magnetic domains are characterized by magnetic force microscopy (MFM). Comparison of PFM and EFM results suggests that the proposed ferroelectricity in LuFe2O4 is not of usual displacive type but of electronic origin. Simultaneous characterization of ferroelectric/charge order and magnetic domains by EFM and MFM, respectively, on the same surface of LuFe2O4 reveals that both domains have irregular patterns of similar shape, but the length scales are quite different. The domain size is approximately 100 nm for the ferroelectric domains, while the magnetic domain size is much larger and gets as large as 1 μm. We also demonstrate that the origin of the formation of irregular domains in LuFe2O4 is not extrinsic but intrinsic.",
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Charge ordering, ferroelectric, and magnetic domains in LuFe2O4 observed by scanning probe microscopy. / Yang, I. K.; Kim, Jeehoon; Lee, S. H.; Cheong, Sang-Wook; Jeong, Y. H.

In: Applied Physics Letters, Vol. 106, No. 15, 152902, 13.04.2015.

Research output: Contribution to journalArticle

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AU - Yang, I. K.

AU - Kim, Jeehoon

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AU - Cheong, Sang-Wook

AU - Jeong, Y. H.

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