Metal-polymer-metal split-dipole nanoantennas

Deirdre M. O'Carroll; James S. Fakonas; Dennis M. Callahan; Martin Schierhorn; Harry A. Atwater

doi:10.1002/adma.201103396

Metal-polymer-metal split-dipole nanoantennas

Deirdre M. O'Carroll, James S. Fakonas, Dennis M. Callahan, Martin Schierhorn, Harry A. Atwater

School of Engineering, Materials Science & Engineering

Research output: Contribution to journal › Article › peer-review

23 Scopus citations

Abstract

The conjugated polymer semiconductor poly(3-hexylthiophene), (P3HT), is integrated directly into the slot region of resonant plasmonic split-dipole nanoantennas. The P3HT radiative emission rate is enhanced by a factor of up to 29, in experiment, and 550 for the ideal case, due to the large local density of optical states in the nanoantenna slot region. Additionally, the theoretical modified luminescence quantum efficiency is shown to increase from 1% to 45% for optimized nanoantenna parameters.

Original language	English (US)
Pages (from-to)	OP136-OP142
Journal	Advanced Materials
Volume	24
Issue number	23
DOIs	https://doi.org/10.1002/adma.201103396
State	Published - Jun 19 2012

All Science Journal Classification (ASJC) codes

Materials Science(all)
Mechanics of Materials
Mechanical Engineering

Keywords

conjugated polymers
nanoantennas
polythiophene
quantum efficiency
radiative emission

Access to Document

10.1002/adma.201103396

Cite this

@article{31645419e5624d5ca9ddc438e8b9ebf9,

title = "Metal-polymer-metal split-dipole nanoantennas",

abstract = "The conjugated polymer semiconductor poly(3-hexylthiophene), (P3HT), is integrated directly into the slot region of resonant plasmonic split-dipole nanoantennas. The P3HT radiative emission rate is enhanced by a factor of up to 29, in experiment, and 550 for the ideal case, due to the large local density of optical states in the nanoantenna slot region. Additionally, the theoretical modified luminescence quantum efficiency is shown to increase from 1% to 45% for optimized nanoantenna parameters.",

keywords = "conjugated polymers, nanoantennas, polythiophene, quantum efficiency, radiative emission",

author = "O'Carroll, {Deirdre M.} and Fakonas, {James S.} and Callahan, {Dennis M.} and Martin Schierhorn and Atwater, {Harry A.}",

year = "2012",

month = jun,

day = "19",

doi = "10.1002/adma.201103396",

language = "English (US)",

volume = "24",

pages = "OP136--OP142",

journal = "Advanced Materials",

issn = "0935-9648",

publisher = "Wiley-VCH Verlag",

number = "23",

}

TY - JOUR

T1 - Metal-polymer-metal split-dipole nanoantennas

AU - O'Carroll, Deirdre M.

AU - Fakonas, James S.

AU - Callahan, Dennis M.

AU - Schierhorn, Martin

AU - Atwater, Harry A.

PY - 2012/6/19

Y1 - 2012/6/19

N2 - The conjugated polymer semiconductor poly(3-hexylthiophene), (P3HT), is integrated directly into the slot region of resonant plasmonic split-dipole nanoantennas. The P3HT radiative emission rate is enhanced by a factor of up to 29, in experiment, and 550 for the ideal case, due to the large local density of optical states in the nanoantenna slot region. Additionally, the theoretical modified luminescence quantum efficiency is shown to increase from 1% to 45% for optimized nanoantenna parameters.

AB - The conjugated polymer semiconductor poly(3-hexylthiophene), (P3HT), is integrated directly into the slot region of resonant plasmonic split-dipole nanoantennas. The P3HT radiative emission rate is enhanced by a factor of up to 29, in experiment, and 550 for the ideal case, due to the large local density of optical states in the nanoantenna slot region. Additionally, the theoretical modified luminescence quantum efficiency is shown to increase from 1% to 45% for optimized nanoantenna parameters.

KW - conjugated polymers

KW - nanoantennas

KW - polythiophene

KW - quantum efficiency

KW - radiative emission

UR - http://www.scopus.com/inward/record.url?scp=84862174541&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=84862174541&partnerID=8YFLogxK

U2 - 10.1002/adma.201103396

DO - 10.1002/adma.201103396

M3 - Article

C2 - 22447722

AN - SCOPUS:84862174541

SN - 0935-9648

VL - 24

SP - OP136-OP142

JO - Advanced Materials

JF - Advanced Materials

IS - 23

ER -

Metal-polymer-metal split-dipole nanoantennas

Abstract

All Science Journal Classification (ASJC) codes

Keywords

Access to Document

Other files and links

Fingerprint

Cite this