Relationship between weak ferromagnetism, superconductivity, and lattice parameter in the A2-x-yBxCeyCuO4 (A,B≡La, Pr, Nd, Sm, Eu, Gd, Y) compounds

T. Schultz, R. Smith, A. Fondado, C. Maley, T. Beacom, P. Tinklenberg, J. Gross, C. Saylor, S. Oseroff, Z. Fisk, S. W. Cheong, T. E. Jones

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Abstract

We report the results obtained by x-ray, dc magnetization, ac magnetic susceptibility, microwave magnetic absorption, and electron paramagnetic resonance of the magnetic and superconductive properties of a large series of compounds of the form A2-x-yBxCeyCuO 4 with A,B≡La, Pr, Nd, Sm, Eu, Gd, and Y. For y=0 antiferromagnetic ordering of the copper moments is present at T N≊280 K for all the compounds formed in the tetragonal T' phase. Weak ferromagnetism (WF) associated with the canting of the copper moments is observed in all the compounds with a lattice parameter, a<a0, a0≊3.91 Å, regardless of the rare-earth (R) ions present in the system. Superconductivity is observed only in the Ce-doped compounds with a≳a1, a1≊3.92 Å. The maximum onset temperature Tc is found for a≊3.95 Å. A phase diagram was obtained by varying the lattice parameter size as a function of A, B, and x. The correlation between the appearance of WF in the undoped compounds and the disappearance of superconductivity in the Ce-doped systems is discussed.

Original languageEnglish (US)
Pages (from-to)6723-6725
Number of pages3
JournalJournal of Applied Physics
Volume75
Issue number10
DOIs
StatePublished - 1994

All Science Journal Classification (ASJC) codes

  • Physics and Astronomy(all)

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